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چکیده
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It is thought that nature already exploits quantum mechanical properties to increase the efficiency of solar
energy harvesting devices. Thus, the operation of these devices can be enhanced by clever design of a
nanoscopic, quantum mechanical system where the quantum coherence plays a crucial role in this process.
In this investigation, we develop a donor–acceptor two level trap dipole model converging the key role
of quantum coherence and aggregation effects along with different initial states. Our analysis reveals that
quenching unwanted emissions is achievable by preparing the system in specific initial state under the effect
of optimal spatial aggregation. Interestingly it is observed that characterizing aggregation-induced properties
and quantum effects of bandgap engineering can increase the power enhancement up to 35.87% compared with
classical counterparts. This encouraging trend suggests a promising novel design aspect of nature-mimicking
photovoltaic devices.
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